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Ice-templating holds promise to become a powerful technique to construct high-performance bioinspired materials. Both ice nucleation and growth during the freezing process are crucial for the final architecture of the ice-templated material. However, effective ways to control these two very important factors are still lacking. Here, we demonstrate that successive ice nucleation and preferential growth can be realized by introducing a wettability gradient on a cold finger. A bulk porous material with a long-range lamellar pattern was obt