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9 kcal mol-1.[Ni2-H2NC(=O)C5H4N2(H2O)2][Ni2,6-(O2C)2C5H3N2]·4.67H2O, a new complex salt containing a bis(2,6-dicarboxypyridine)nickel(II) anion and a bis(2-amidopyridine)diaquanickel(II) cation, was synthesized and characterized. The crystal is stabilized by an extensive network of hydrogen bonds. Alternate layers of anions and cations/water molecules parallel to (01 can be distinguished. Computational studies of the network packing of the title compound by high-level DFT-D/B3LYP calculations indicate stabilization of the networks with
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