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The results showed that the right level of Ni addition can effectively modulate the physicochemical properties of MCM-41. For a Ni running of 25.1 wt % (Cat-C), the catalyst showed an optimal catalytic performance, a decrease into the percentage of oxygenated compounds within the product from 35.6 (MCM-41) to 13.4per cent, and an increase in the relative complete number of olefins plus aromatics from 62.2 (MCM-41) to 84.6%. The wonderful catalytic performance o