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Ni-Co alloy catalyst (10% Ni-5% Co/Al-MCM48) triggered the greatest H2 (∼52 vol%) selectivity as a result of enhanced Ni dispersion and synergy effect between Ni and Co. Moreover, the application of bi-metal alloy on Al-MCM48 showed no coke formation and considerably decreased CO2 and hydrocarbon selectivity into the product fuel. Overall, this study introduced a promising answer for sewage sludge disposal when it comes to clean H2 gener