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Vapor wall losses can affect the yields of secondary organic aerosol. The effects of surface-to-volume (S/V) ratio and relative humidity (RH) on the vapor-wall interactions were investigated in this study. The oxygenated volatile organic compounds (OVOCs) were generated from toluene-H2O2 irradiations. The average gas to wall loss rate constant (kgw) of OVOCs in a 400 L reactor (S/V = 7.5 m-1) is 2.47 (2.41 under humid conditions) times higher than that in a 5000 L reactor (S/V = 3.6 m-1) under dry conditions. In contrast, the average de
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