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Volatile binary liquid samples on wetting substrates are known to undergo either spreading or contraction tendencies, as a result of solutal Marangoni stresses due to differential volatility. Enhanced spreading is commonly thought to occur when the lower surface tension component is more 'volatile', while contraction is expected otherwise. We seek to test the limits of this scenario for various configurations such as sessile drops with free or pinned contact lines, without or with microparticles, and tears-of-wine menisci. We consider
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